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Author Hase, Muneaki; Katsuragawa, Masayuki; Constantinescu, Anca Monia; Petek, Hrvoje openurl 
  Title Frequency comb generation at terahertz frequencies by coherent phonon excitation in silicon Type Journal Article
  Year 2012 Publication Nature Photonics Abbreviated Journal (down) Nat. Photon.  
  Volume 6 Issue Pages 243–247  
  Keywords fromIPMRAS  
  Abstract High-order nonlinear light–matter interactions in gases enable the generation of X-ray and attosecond light pulses, metrology and spectroscopy1. Optical nonlinearities in solid-state materials are particularly interesting for combining optical and electronic functions for high-bandwidth information processing2. Third-order nonlinear optical processes in silicon have been used to process optical signals with bandwidths greater than 1 GHz (ref. 2). However, fundamental physical processes for a silicon-based optical modulator in the terahertz bandwidth range have not yet been explored. Here, we demonstrate ultrafast phononic modulation of the optical index of silicon by irradiation with intense few-cycle femtosecond pulses. The anisotropic reflectivity modulation by the resonant Raman susceptibility at the fundamental frequency of the longitudinal optical phonon of silicon (15.6 THz) generates a frequency comb up to seventh order. All-optical >100 THz frequency comb generation is realized by harnessing the coherent atomic motion of the silicon crystalline lattice at its highest mechanical frequency.  
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  Call Number RPLAB @ gujma @ Serial 794  
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Author Bonifas, Andrew P.; McCreery, Richard L. openurl 
  Title ‘Soft’ Au, Pt and Cu contacts for molecular junctions through surface-diffusion-mediated deposition Type Journal Article
  Year 2010 Publication Nature Nanotechnology Abbreviated Journal (down) Nat. Nanotech.  
  Volume 5 Issue 8 Pages 612–617  
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  Abstract Virtually all types of molecular electronic devices depend on electronically addressing a molecule or molecular layer through the formation of a metallic contact. The introduction of molecular devices into integrated circuits will probably depend on the formation of contacts using a vapour deposition technique, but this approach frequently results in the metal atoms penetrating or damaging the molecular layer. Here, we report a method of forming 'soft' metallic contacts on molecular layers through surface-diffusion-mediated deposition, in which the metal atoms are deposited remotely and then diffuse onto the molecular layer, thus eliminating the problems of penetration and damage. Molecular junctions fabricated by this method exhibit excellent yield (typically >90%) and reproducibility, and allow examination of the effects of molecular-layer structure, thickness and contact work function.  
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  Call Number RPLAB @ gujma @ Serial 682  
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Author Freer, Erik M.; Grachev, Oleg; Duan, Xiangfeng; Martin, Samuel; Stumbo, David P. openurl 
  Title High-yield self-limiting single-nanowire assembly with dielectrophoresis Type Journal Article
  Year 2010 Publication Nature Nanotechnology Abbreviated Journal (down) Nat. Nanotech.  
  Volume 5 Issue 7 Pages 525–530  
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  Abstract Single-crystal nanowire transistors and other nanowire-based devices could have applications in large-area and flexible electronics if conventional top-down fabrication techniques can be integrated with high-precision bottom-up nanowire assembly. Here, we extend dielectrophoretic nanowire assembly to achieve a 98.5% yield of single nanowires assembled over 16,000 patterned electrode sites with submicrometre alignment precision. The balancing of surface, hydrodynamic and dielectrophoretic forces makes the self-assembly process controllable, and a hydrodynamic force component makes it self-limiting. Our approach represents a methodology to quantify nanowire assembly, and makes single nanowire assembly possible over an area limited only by the ability to reproduce process conditions uniformly.  
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  Call Number RPLAB @ gujma @ Serial 683  
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Author Konstantatos, Gerasimos; Sargent, Edward H. openurl 
  Title Nanostructured materials for photon detection Type Journal Article
  Year 2010 Publication Nature Nanotechnology Abbreviated Journal (down) Nat. Nanotech.  
  Volume 5 Issue 6 Pages 391–400  
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  Abstract The detection of photons underpins imaging, spectroscopy, fibre-optic communications and time-gated distance measurements. Nanostructured materials are attractive for detection applications because they can be integrated with conventional silicon electronics and flexible, large-area substrates, and can be processed from the solution phase using established techniques such as spin casting, spray coating and layer-by-layer deposition. In addition, their performance has improved rapidly in recent years. Here we review progress in light sensing using nanostructured materials, focusing on solution-processed materials such as colloidal quantum dots and metal nanoparticles. These devices exhibit phenomena such as absorption of ultraviolet light, plasmonic enhancement of absorption, size-based spectral tuning, multiexciton generation, and charge carrier storage in surface and interface traps.  
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  Call Number RPLAB @ gujma @ Serial 684  
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Author Peruzzo, Alberto; Laing, Anthony; Politi, Alberto; Rudolph, Terry; O'Brien, Jeremy L. openurl 
  Title Multimode quantum interference of photons in multiport integrated devices Type Journal Article
  Year 2011 Publication Nature Communications Abbreviated Journal (down) Nat. Comm.  
  Volume 2 Issue 224 Pages 6  
  Keywords fromIPMRAS  
  Abstract Photonics is a leading approach in realizing future quantum technologies and recently, optical waveguide circuits on silicon chips have demonstrated high levels of miniaturization and performance. Multimode interference (MMI) devices promise a straightforward implementation of compact and robust multiport circuits. Here, we show quantum interference in a 2×2 MMI coupler with visibility of V=95.6+/-0.9%. We further demonstrate the operation of a 4×4 port MMI device with photon pairs, which exhibits complex quantum interference behaviour. We have developed a new technique to fully characterize such multiport devices, which removes the need for phase-sensitive measurements and may find applications for a wide range of photonic devices. Our results show that MMI devices can operate in the quantum regime with high fidelity and promise substantial simplification and concatenation of photonic quantum circuits.  
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  Call Number RPLAB @ gujma @ Serial 763  
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Author Ikuta, Rikizo; Kusaka, Yoshiaki; Kitano, suyoshi; Kato, Hiroshi; Yamamoto, Takashi; Koashi, Masato; Imoto, Nobuyuki openurl 
  Title Wide-band quantum interface for visible-totelecommunication wavelength conversion Type Journal Article
  Year 2011 Publication Nature Communications Abbreviated Journal (down) Nat. Comm.  
  Volume 2 Issue Pages 5  
  Keywords fromIPMRAS  
  Abstract Although near-infrared photons in telecommunication bands are required for long-distance quantum communication, various quantum information tasks have been performed by using visible photons for the past two decades. Recently, such visible photons from diverse media including atomic quantum memories have also been studied. Optical frequency down-conversion from visible to telecommunication bands while keeping the quantum states is thus required for bridging such wavelength gaps. Here we report demonstration of a quantum interface of frequency down-conversion from visible to telecommunication bands by using a nonlinear crystal, which has a potential to work over wide bandwidths, leading to a high-speed interface of frequency conversion. We achieved the conversion of a picosecond visible photon at 780 nm to a 1,522-nm photon, and observed that the conversion process retained entanglement between the down-converted photon and another photon.  
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  Call Number RPLAB @ gujma @ Serial 764  
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Author Crespi, Andrea; Ramponi, Roberta; Osellame, Roberto; Sansoni, Linda; Bongioanni, Irene; Sciarrino, Fabio; Vallone, Giuseppe; Mataloni, Paolo openurl 
  Title Integrated photonic quantum gates for polarization qubits Type Journal Article
  Year 2011 Publication Nature Communications Abbreviated Journal (down) Nat. Comm.  
  Volume 2 Issue 566 Pages 6  
  Keywords fromIPMRAS  
  Abstract The ability to manipulate quantum states of light by integrated devices may open new perspectives both for fundamental tests of quantum mechanics and for novel technological applications. However, the technology for handling polarization-encoded qubits, the most commonly adopted approach, is still missing in quantum optical circuits. Here we demonstrate the first integrated photonic controlled-NOT (CNOT) gate for polarization-encoded qubits. This result has been enabled by the integration, based on femtosecond laser waveguide writing, of partially polarizing beam splitters on a glass chip. We characterize the logical truth table of the quantum gate demonstrating its high fidelity to the expected one. In addition, we show the ability of this gate to transform separable states into entangled ones and vice versa. Finally, the full accessibility of our device is exploited to carry out a complete characterization of the CNOT gate through a quantum process tomography.  
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  Call Number RPLAB @ gujma @ Serial 765  
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Author Berlín, Guido; Brassard, Gilles; Bussières, Félix; Godbout, Nicolas; Slater, Joshua A.; Tittel, Wolfgang openurl 
  Title Experimental loss-tolerant quantum coin flipping Type Journal Article
  Year 2011 Publication Nature Communications Abbreviated Journal (down) Nat. Comm.  
  Volume 2 Issue 561 Pages 7  
  Keywords fromIPMRAS  
  Abstract Coin flipping is a cryptographic primitive in which two distrustful parties wish to generate a random bit to choose between two alternatives. This task is impossible to realize when it relies solely on the asynchronous exchange of classical bits: one dishonest player has complete control over the final outcome. It is only when coin flipping is supplemented with quantum communication that this problem can be alleviated, although partial bias remains. Unfortunately, practical systems are subject to loss of quantum data, which allows a cheater to force a bias that is complete or arbitrarily close to complete in all previous protocols and implementations. Here we report on the first experimental demonstration of a quantum coin-flipping protocol for which loss cannot be exploited to cheat better. By eliminating the problem of loss, which is unavoidable in any realistic setting, quantum coin flipping takes a significant step towards real-world applications of quantum communication.  
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  Call Number RPLAB @ gujma @ Serial 766  
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Author Knee, George C.; Simmons, Stephanie; Gauger, Erik M.; Morton, John J. L.; Riemann, Helge; Abrosimov, Nikolai V.; Becker, Peter; Pohl, Hans-Joachim; Itoh, Kohei M.; Thewalt, Mike L. W.; Briggs, G. Andrew D.; Benjamin, Simon C. openurl 
  Title Violation of a Leggett–Garg inequality with ideal non-invasive measurements Type Journal Article
  Year 2012 Publication Nature Communications Abbreviated Journal (down) Nat. Comm.  
  Volume 3 Issue 606 Pages 6  
  Keywords fromIPMRAS  
  Abstract The quantum superposition principle states that an entity can exist in two different states simultaneously, counter to our 'classical' intuition. Is it possible to understand a given system's behaviour without such a concept? A test designed by Leggett and Garg can rule out this possibility. The test, originally intended for macroscopic objects, has been implemented in various systems. However to date no experiment has employed the 'ideal negative result' measurements that are required for the most robust test. Here we introduce a general protocol for these special measurements using an ancillary system, which acts as a local measuring device but which need not be perfectly prepared. We report an experimental realization using spin-bearing phosphorus impurities in silicon. The results demonstrate the necessity of a non-classical picture for this class of microscopic system. Our procedure can be applied to systems of any size, whether individually controlled or in a spatial ensemble.  
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  Call Number RPLAB @ gujma @ Serial 767  
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Author Smith, Devin H.; Gillett, Geoff; de Almeida, Marcelo P.; Branciard, Cyril; Fedrizzi, Alessandro; Weinhold, Till J.; Lita, Adriana; Calkins, Brice; Gerrits, Thomas; Wiseman, Howard M.; Nam, Sae Woo; White, Andrew G. openurl 
  Title Conclusive quantum steering with superconducting transition-edge sensors Type Journal Article
  Year 2012 Publication Nature Communications Abbreviated Journal (down) Nat. Comm.  
  Volume 3 Issue 625 Pages 6  
  Keywords fromIPMRAS  
  Abstract Quantum steering allows two parties to verify shared entanglement even if one measurement device is untrusted. A conclusive demonstration of steering through the violation of a steering inequality is of considerable fundamental interest and opens up applications in quantum communication. To date, all experimental tests with single-photon states have relied on post selection, allowing untrusted devices to cheat by hiding unfavourable events in losses. Here we close this 'detection loophole' by combining a highly efficient source of entangled photon pairs with superconducting transition-edge sensors. We achieve an unprecedented ~62% conditional detection efficiency of entangled photons and violate a steering inequality with the minimal number of measurement settings by 48 s.d.s. Our results provide a clear path to practical applications of steering and to a photonic loophole-free Bell test.  
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  Call Number RPLAB @ gujma @ Serial 768  
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