Abstract: High-order nonlinear light–matter interactions in gases enable the generation of X-ray and attosecond light pulses, metrology and spectroscopy1. Optical nonlinearities in solid-state materials are particularly interesting for combining optical and electronic functions for high-bandwidth information processing2. Third-order nonlinear optical processes in silicon have been used to process optical signals with bandwidths greater than 1 GHz (ref. 2). However, fundamental physical processes for a silicon-based optical modulator in the terahertz bandwidth range have not yet been explored. Here, we demonstrate ultrafast phononic modulation of the optical index of silicon by irradiation with intense few-cycle femtosecond pulses. The anisotropic reflectivity modulation by the resonant Raman susceptibility at the fundamental frequency of the longitudinal optical phonon of silicon (15.6 THz) generates a frequency comb up to seventh order. All-optical >100 THz frequency comb generation is realized by harnessing the coherent atomic motion of the silicon crystalline lattice at its highest mechanical frequency.

Abstract: In the same way that micro-mechanical resonators resemble guitar strings and drums, surface acoustic waves resemble the sound these instruments produce, but moving over a solid surface rather than through air. In contrast with oscillations in suspended resonators, such propagating mechanical waves have not before been studied near the quantum mechanical limits. Here, we demonstrate local probing of surface acoustic waves with a displacement sensitivity of 30amRMSHz-1/2 and detection sensitivity on the single-phonon level after averaging, at a frequency of 932MHz. Our probe is a piezoelectrically coupled single-electron transistor, which is sufficiently fast, non-destructive and localized to enable us to track pulses echoing back and forth in a long acoustic cavity, self-interfering and ringing the cavity up and down. We project that strong coupling to quantum circuits will enable new experiments, and hybrids using the unique features of surface acoustic waves. Prospects include quantum investigations of phonon-phonon interactions, and acoustic coupling to superconducting qubits for which we present favourable estimates.

Abstract: Optical random-access memory (o-RAM) has been regarded as one of the most difficult challenges in terms of replacing its various functionalities in electronic circuitry with their photonic counterparts. Nevertheless, it constitutes a key device in optical routing and processing. Here, we demonstrate that photonic crystal nanocavities with an ultrasmall buried heterostructure design can solve most of the problems encountered in previous o-RAMs. By taking advantage of the strong confinement of photons and carriers and allowing heat to escape efficiently, we have realized all-optical RAMs with a power consumption of only 30 nW, which is more than 300 times lower than the previous record, and have achieved continuous operation. We have also demonstrated their feasibility in multibit integration. This paves the way for constructing a low-power large-scale o-RAM system that can handle high-bit-rate optical signals.

Abstract: Quantum networks must have the crucial ability to entangle quantum nodes. A prominent example is the quantum repeater, which allows the distance barrier of direct transmission of single photons to be overcome, provided remote quantum memories can be entangled in a heralded fashion. Here, we report the observation of heralded entanglement between two ensembles of rare-earth ions doped into separate crystals. A heralded single photon is sent through a 50/50 beamsplitter, creating a single-photon entangled state delocalized between two spatial modes. The quantum state of each mode is subsequently mapped onto a crystal, leading to an entangled state consisting of a single collective excitation delocalized between two crystals. This entanglement is revealed by mapping it back to optical modes and by estimating the concurrence of the retrieved light state. Our results highlight the potential of crystals doped with rare-earth ions for entangled quantum nodes and bring quantum networks based on solid-state resources one step closer.

Abstract: Quantum steering allows two parties to verify shared entanglement even if one measurement device is untrusted. A conclusive demonstration of steering through the violation of a steering inequality is of considerable fundamental interest and opens up applications in quantum communication. To date, all experimental tests with single-photon states have relied on post selection, allowing untrusted devices to cheat by hiding unfavourable events in losses. Here we close this 'detection loophole' by combining a highly efficient source of entangled photon pairs with superconducting transition-edge sensors. We achieve an unprecedented ~62% conditional detection efficiency of entangled photons and violate a steering inequality with the minimal number of measurement settings by 48 s.d.s. Our results provide a clear path to practical applications of steering and to a photonic loophole-free Bell test.