Abstract: Recent advancements in metamaterials and plasmonics have promised a number of exciting applications, in particular at terahertz and optical frequencies. Unfortunately, the noble metals used in these photonic structures are not particularly good conductors at high frequencies, resulting in significant dissipative loss. Here, we address the question of what is a good conductor for metamaterials and plasmonics. For resonant metamaterials, we develop a figure-of-merit for conductors that allows for a straightforward classification of conducting materials according to the resulting dissipative loss in the metamaterial. Application of our method predicts that graphene and high-Tc superconductors are not viable alternatives for metals in metamaterials. We also provide an overview of a number of transition metals, alkali metals and transparent conducting oxides. For plasmonic systems, we predict that graphene and high-Tc superconductors cannot outperform gold as a platform for surface plasmon polaritons, because graphene has a smaller propagation length-to-wavelength ratio.

Abstract: Quantum networks must have the crucial ability to entangle quantum nodes. A prominent example is the quantum repeater, which allows the distance barrier of direct transmission of single photons to be overcome, provided remote quantum memories can be entangled in a heralded fashion. Here, we report the observation of heralded entanglement between two ensembles of rare-earth ions doped into separate crystals. A heralded single photon is sent through a 50/50 beamsplitter, creating a single-photon entangled state delocalized between two spatial modes. The quantum state of each mode is subsequently mapped onto a crystal, leading to an entangled state consisting of a single collective excitation delocalized between two crystals. This entanglement is revealed by mapping it back to optical modes and by estimating the concurrence of the retrieved light state. Our results highlight the potential of crystals doped with rare-earth ions for entangled quantum nodes and bring quantum networks based on solid-state resources one step closer.

Abstract: Optical random-access memory (o-RAM) has been regarded as one of the most difficult challenges in terms of replacing its various functionalities in electronic circuitry with their photonic counterparts. Nevertheless, it constitutes a key device in optical routing and processing. Here, we demonstrate that photonic crystal nanocavities with an ultrasmall buried heterostructure design can solve most of the problems encountered in previous o-RAMs. By taking advantage of the strong confinement of photons and carriers and allowing heat to escape efficiently, we have realized all-optical RAMs with a power consumption of only 30 nW, which is more than 300 times lower than the previous record, and have achieved continuous operation. We have also demonstrated their feasibility in multibit integration. This paves the way for constructing a low-power large-scale o-RAM system that can handle high-bit-rate optical signals.

Abstract: High-order nonlinear light–matter interactions in gases enable the generation of X-ray and attosecond light pulses, metrology and spectroscopy1. Optical nonlinearities in solid-state materials are particularly interesting for combining optical and electronic functions for high-bandwidth information processing2. Third-order nonlinear optical processes in silicon have been used to process optical signals with bandwidths greater than 1 GHz (ref. 2). However, fundamental physical processes for a silicon-based optical modulator in the terahertz bandwidth range have not yet been explored. Here, we demonstrate ultrafast phononic modulation of the optical index of silicon by irradiation with intense few-cycle femtosecond pulses. The anisotropic reflectivity modulation by the resonant Raman susceptibility at the fundamental frequency of the longitudinal optical phonon of silicon (15.6 THz) generates a frequency comb up to seventh order. All-optical >100 THz frequency comb generation is realized by harnessing the coherent atomic motion of the silicon crystalline lattice at its highest mechanical frequency.

Abstract: Existing infrared detectors rely on complex microfabrication and thermal management methods. Here, we report an attractive platform of low-thermal-mass resonators inspired by the architectures of iridescent Morpho butterfly scales. In these resonators, the optical cavity is modulated by its thermal expansion and refractive index change, resulting in `wavelength conversion' of mid-wave infrared (3-8 µm) radiation into visible iridescence changes. By doping Morpho butterfly scales with single-walled carbon nanotubes, we achieved mid-wave infrared detection with 18-62 mK noise-equivalent temperature difference and 35-40 Hz heat-sink-free response speed. The nanoscale pitch and the extremely small thermal mass of individual `pixels' promise significant improvements over existing detectors. Computational analysis explains the origin of this thermal response and guides future conceptually new bio-inspired thermal imaging sensor designs.

Abstract: Emission from a resonantly excited quantum emitter is a fascinating research topic within the field of quantum optics and is a useful source for different types of quantum light fields. The resonance spectrum consists of a single spectral line that develops into a triplet above saturation of the quantum emitter. The three closely spaced photon channels from the resonance fluorescence have different photon statistical signatures. We present a detailed photon statistics analysis of the resonance fluorescence emission triplet from a solid-state-based artificial atom, that is, a semiconductor quantum dot. The photon correlation measurements demonstrate both `single' and `cascaded' photon emission from the Mollow triplet sidebands. The bright and narrow sideband emission (5.9 × 106 photons per second into the first lens) can be conveniently frequency-tuned by laser detuning over 15 times its linewidth (Δv ~ 1.0 GHz). These unique properties make the Mollow triplet sideband emission a valuable light source for quantum light spectroscopy and quantum information applications, for example.

Abstract: A new asynchronous coherent optical sampling method allows for the direct visualization of actively mode-locked quantum cascade laser pulses at terahertz wavelengths.