Abstract: High-order nonlinear light–matter interactions in gases enable the generation of X-ray and attosecond light pulses, metrology and spectroscopy1. Optical nonlinearities in solid-state materials are particularly interesting for combining optical and electronic functions for high-bandwidth information processing2. Third-order nonlinear optical processes in silicon have been used to process optical signals with bandwidths greater than 1 GHz (ref. 2). However, fundamental physical processes for a silicon-based optical modulator in the terahertz bandwidth range have not yet been explored. Here, we demonstrate ultrafast phononic modulation of the optical index of silicon by irradiation with intense few-cycle femtosecond pulses. The anisotropic reflectivity modulation by the resonant Raman susceptibility at the fundamental frequency of the longitudinal optical phonon of silicon (15.6 THz) generates a frequency comb up to seventh order. All-optical >100 THz frequency comb generation is realized by harnessing the coherent atomic motion of the silicon crystalline lattice at its highest mechanical frequency.

Abstract: Existing infrared detectors rely on complex microfabrication and thermal management methods. Here, we report an attractive platform of low-thermal-mass resonators inspired by the architectures of iridescent Morpho butterfly scales. In these resonators, the optical cavity is modulated by its thermal expansion and refractive index change, resulting in `wavelength conversion' of mid-wave infrared (3-8 µm) radiation into visible iridescence changes. By doping Morpho butterfly scales with single-walled carbon nanotubes, we achieved mid-wave infrared detection with 18-62 mK noise-equivalent temperature difference and 35-40 Hz heat-sink-free response speed. The nanoscale pitch and the extremely small thermal mass of individual `pixels' promise significant improvements over existing detectors. Computational analysis explains the origin of this thermal response and guides future conceptually new bio-inspired thermal imaging sensor designs.

Abstract: Emission from a resonantly excited quantum emitter is a fascinating research topic within the field of quantum optics and is a useful source for different types of quantum light fields. The resonance spectrum consists of a single spectral line that develops into a triplet above saturation of the quantum emitter. The three closely spaced photon channels from the resonance fluorescence have different photon statistical signatures. We present a detailed photon statistics analysis of the resonance fluorescence emission triplet from a solid-state-based artificial atom, that is, a semiconductor quantum dot. The photon correlation measurements demonstrate both `single' and `cascaded' photon emission from the Mollow triplet sidebands. The bright and narrow sideband emission (5.9 × 106 photons per second into the first lens) can be conveniently frequency-tuned by laser detuning over 15 times its linewidth (Δv ~ 1.0 GHz). These unique properties make the Mollow triplet sideband emission a valuable light source for quantum light spectroscopy and quantum information applications, for example.

Abstract: A new asynchronous coherent optical sampling method allows for the direct visualization of actively mode-locked quantum cascade laser pulses at terahertz wavelengths.