|
Lieberzeit, P., Afzal, A., Rehman, A., & Dickert, F. (2007). Nanoparticles for detecting pollutants and degradation processes with mass-sensitive sensors. Sensors and Actuators B: Chemical, 127(1), 132–136.
Abstract: Compared with thin films, nanoparticle layers as coatings for QCM offer substantially increased interaction areas and sensitivities with favourable response times. Molybdenum disulphide (MoS2), e.g. has turned out to be a highly suitable material for interacting with thiols. The resulting materials are sufficiently soft according to Pearson to bind sulphur containing compounds reversibly. Depositing MoS2 nanoparticle submonolayers (particle size 200–300 nm) leads to an increase in sensor response by a factor of ten compared to a pure gold layer. Additionally, the nanoparticle layers show fully reversible sensor signals. Particle synthesis can also be combined with the molecular imprinting approach: by a precipitation technique, it is possible to generate molecularly imprinted TiO2 particles for engine oil degradation measurements. Compared with deposited thin layers, particles incorporate oxidised compounds from lubricants by a factor of two better.
|
|
|
Lu, C. - Y., Zhou, X. - Q., Gühne, O., Gao, W. - B., Zhang, J., Yuan, Z. - S., et al. (2007). Experimental entanglement of six photons in graph states. Nat. Phys., 3(2), 91–95.
Abstract: Graph states-multipartite entangled states that can be represented by mathematical graphs-are important resources for quantum computation, quantum error correction, studies of multiparticle entanglement and fundamental tests of non-locality and decoherence. Here, we demonstrate the experimental entanglement of six photons and engineering of multiqubit graph states. We have created two important examples of graph states, a six-photon Greenberger-Horne-Zeilinger state, the largest photonic Schrödinger cat so far, and a six-photon cluster state, a state-of-the-art `one-way quantum computer'. With small modifications, our method allows us, in principle, to create various further graph states, and therefore could open the way to experimental tests of, for example, quantum algorithms or loss- and fault-tolerant one-way quantum computation.
|
|
|
Bell, M., Kaurova, N., Divochiy, A., Gol'tsman, G., Bird, J., Sergeev, A., et al. (2007). On the nature of resistive transition in disordered superconducting nanowires. IEEE Trans. Appl. Supercond., 17(2), 267–270.
Abstract: Hot-electron single-photon counters based on long superconducting nanowires are starting to become popular in optical and infrared technologies due to their ultimately high sensitivity and very high response speed. We investigate intrinsic fluctuations in long NbN nanowires in the temperature range of 4.2 K-20 K, i.e. above and below the superconducting transition. These fluctuations are responsible for fluctuation resistivity and also determine the noise in practical devices. Measurements of the fluctuation resistivity were performed at low current densities and also in external magnetic fields up to 5 T. Above the BCS critical temperature T co the resistivity is well described by the Aslamazov-Larkin (AL) theory for two-dimensional samples. Below T co the measured resistivity is in excellent agreement with the Langer-Ambegaokar-McCumber-Halperin (LAMH) theory developed for one-dimensional superconductors. Despite that our nanowires of 100 nm width are two-dimensional with respect to the coherence length, our analysis shows that at relatively low current densities the one-dimensional LAMH mechanism based on thermally induced phase slip centers dominates over the two-dimensional mechanism related to unbinding of vortex-antivortex pairs below the Berezinskii-Kosterlitz-Thouless transition.
|
|
|
Novotny, L. (2007). Effective wavelength scaling for optical antennas. Phys. Rev. Lett., 98(26), 266802(1–4).
Abstract: In antenna theory, antenna parameters are directly related to the wavelength λ of incident radiation, but this scaling fails at optical frequencies where metals behave as strongly coupled plasmas. In this Letter we show that antenna designs can be transferred to the optical frequency regime by replacing λ by a linearly scaled effective wavelength λeff=n1+n2λ/λp, with λp being the plasma wavelength and n1, n2 being coefficients that depend on geometry and material properties. It is assumed that the antenna is made of linear segments with radii Râ‰<aa>λ. Optical antennas hold great promise for increasing the efficiency of photovoltaics, light-emitting devices, and optical sensors.
|
|
|
Huard, B., Pothier, H., Esteve, D., & Nagaev, K. E. (2007). Electron heating in metallic resistors at sub-Kelvin temperature. Phys. Rev. B, 76, 165426(1–9).
Abstract: In the presence of Joule heating, the electronic temperature in a metallic resistor placed at sub-Kelvin temperatures can significantly exceed the phonon temperature. Electron cooling proceeds mainly through two processes: electronic diffusion to and from the connecting wires and electron-phonon coupling. The goal of this paper is to present a general solution of the problem in a form that can easily be used in practical situations. As an application, we compute two quantities that depend on the electronic temperature profile: the second and the third cumulant of the current noise at zero frequency, as a function of the voltage across the resistor. We also consider time-dependent heating, an issue relevant for experiments in which current pulses are used, for instance, in time-resolved calorimetry experiments.
|
|