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| Author |
Васильева, И. А.; Компанеец, В. В.; Красная, Ж. А.; Чижикова, З. А. |
| Title |
Проявление внутримолекулярных вибронных взаимодействий в тонкоструктурных спектрах флуоресценции и возбуждения флуоресценции полиеновых δ-диметиламинокетонов |
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Journal Article |
| Year |
2011 |
Publication |
Оптический журнал |
Abbreviated Journal |
Опт. ж. |
| Volume |
78 |
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5 |
Pages |
3-8 |
| Keywords |
спектры флуоресценции; вибрационный анализ; адиабатическое гармоническое приближение; бесфононная линия; фононное крыло |
| Abstract |
Проведен вибрационный анализ спектров флуоресценции и возбуждения флуоресценции, полученных методом Шпольского при 4,2 K. Рассчитаны параметры внутримолекулярных взаимодействий двух δ-диметиламинокетонов. Для определения интегральных интенсивностей вибронных полос в спектрах с тонкой структурой на интенсивном сплошном фоне выполнено моделирование спектров путем представления полосы каждого из вибронных переходов бесфононной линией и фононным крылом с определенными параметрами (полуширинами, фактором Дебая–Валлера). Показано, что нарушение зеркальной симметрии в сопряженных спектрах флуоресценции и возбуждения флуоресценции этих двух соединений может быть обÑŠяснено интерференцией франк-кондоновского и герцберг-теллеровского взаимодействий. |
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RPLAB @ gujma @ |
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Antipov, Andrei; Bell, Matt; Yasar, Mesut; Mitin, Vladimir; Scharmach, William; Swihart, Mark; Verevkin, Aleksandr; Sergeev, Andrei |
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Luminescence of colloidal CdSe/ZnS nanoparticles: high sensitivity to solvent phase transitions |
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Journal Article |
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2011 |
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Nanoscale Research Letters |
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Nan. Res. Lett. |
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6 |
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7 |
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We investigate nanosecond photoluminescence processes in colloidal core/shell CdSe/ZnS nanoparticles dissolved in water and found strong sensitivity of luminescence to the solvent state. Several pronounced changes have been observed in the narrow temperature interval near the water melting point. First of all, the luminescence intensity substantially (approximately 50%) increases near the transition. In a large temperature scale, the energy peak of the photoluminescence decreases with temperature due to temperature dependence of the energy gap. Near the melting point, the peak shows N-type dependence with the maximal changes of approximately 30 meV. The line width increases with temperature and also shows N-type dependence near the melting point. The observed effects are associated with the reconstruction of ligands near the ice/water phase transition. |
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Wiechers, C.; Lydersen, L.; Wittmann, C.; Elser, D.; Skaar, J.; Marquardt, Ch; Makarov, V.; Leuchs, G. |
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After-gate attack on a quantum cryptosystem |
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Journal Article |
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2011 |
Publication |
New J. Phys. |
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13 |
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1 |
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14 |
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quantum cryptography; hacking; interception; attack; SPD; APD; QKD |
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We present a method to control the detection events in quantum key distribution systems that use gated single-photon detectors. We employ bright pulses as faked states, timed to arrive at the avalanche photodiodes outside the activation time. The attack can remain unnoticed, since the faked states do not increase the error rate per se. This allows for an intercept-resend attack, where an eavesdropper transfers her detection events to the legitimate receiver without causing any errors. As a side effect, afterpulses, originating from accumulated charge carriers in the detectors, increase the error rate. We have experimentally tested detectors of the system id3110 (Clavis2) from ID Quantique. We identify the parameter regime in which the attack is feasible despite the side effect. Furthermore, we outline how simple modifications in the implementation can make the device immune to this attack. |
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RPLAB @ gujma @ |
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730 |
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Ожегов, Роман Викторович |
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Флуктуационная чувствительность и стабильность приемников с СИС и HEB смесителями для терагерцового тепловидения |
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2011 |
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Радиофизика |
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135 |
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HEB |
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RPLAB @ gujma @ |
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731 |
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Huang, Kevin C. Y.; Jun, Young Chul; Seo, Min-Kyo; Brongersma, Mark L. |
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Power flow from a dipole emitter near an optical antenna |
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Journal Article |
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2011 |
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Optics Express |
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Opt. Express |
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19 |
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20 |
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19084-19092 |
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optical antennas |
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Current methods to calculate the emission enhancement of a quantum emitter coupled to an optical antenna of arbitrary geometry rely on analyzing the total Poynting vector power flow out of the emitter or the dyadic Green functions from full-field numerical simulations. Unfortunately, these methods do not provide information regarding the nature of the dominant energy decay pathways. We present a new approach that allows for a rigorous separation, quantification, and visualization of the emitter output power flow captured by an antenna and the subsequent reradiation power flow to the far field. Such analysis reveals unprecedented details of the emitter/antenna coupling mechanisms and thus opens up new design strategies for strongly interacting emitter/antenna systems used in sensing, active plasmonics and metamaterials, and quantum optics. |
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RPLAB @ gujma @ |
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743 |
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Hu, Xiaolong; Dauler, Eric A.; Molnar, Richard J.; Berggren, Karl K. |
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Superconducting nanowire single-photon detectors integrated with optical nano-antennae |
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Journal Article |
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2011 |
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Optics Express |
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Opt. Express |
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19 |
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1 |
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17-31 |
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optical antennas |
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Optical nano-antennae have been integrated with semiconductor lasers to intensify light at the nanoscale and photodiodes to enhance photocurrent. In quantum optics, plasmonic metal structures have been used to enhance nonclassical light emission from single quantum dots. Absorption and detection of single photons from free space could also be enhanced by nanometallic antennae, but this has not previously been demonstrated. Here, we use nano-optical transmission effects in a one-dimensional gold structure, combined with optical cavity resonance, to form optical nano-antennae, which are further used to couple single photons from free space into a 80-nm-wide superconducting nanowire. This antenna-assisted coupling enables a superconducting nanowire single-photon detector with 47% device efficiency at the wavelength of 1550 nm and 9-μm-by-9-μm active area while maintaining a reset time of only 5 ns. We demonstrate nanoscale antenna-like structures to achieve exceptional efficiency and speed in single-photon detection. |
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745 |
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Peruzzo, Alberto; Laing, Anthony; Politi, Alberto; Rudolph, Terry; O'Brien, Jeremy L. |
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Multimode quantum interference of photons in multiport integrated devices |
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Journal Article |
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2011 |
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Nature Communications |
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Nat. Comm. |
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2 |
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224 |
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6 |
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fromIPMRAS |
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Photonics is a leading approach in realizing future quantum technologies and recently, optical waveguide circuits on silicon chips have demonstrated high levels of miniaturization and performance. Multimode interference (MMI) devices promise a straightforward implementation of compact and robust multiport circuits. Here, we show quantum interference in a 2×2 MMI coupler with visibility of V=95.6+/-0.9%. We further demonstrate the operation of a 4×4 port MMI device with photon pairs, which exhibits complex quantum interference behaviour. We have developed a new technique to fully characterize such multiport devices, which removes the need for phase-sensitive measurements and may find applications for a wide range of photonic devices. Our results show that MMI devices can operate in the quantum regime with high fidelity and promise substantial simplification and concatenation of photonic quantum circuits. |
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RPLAB @ gujma @ |
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763 |
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Novotny, Lukas; van Hulst, Niek |
| Title |
Antennas for light |
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Journal Article |
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2011 |
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Nature Photonics |
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Nat. Photon. |
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5 |
Issue |
2 |
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83-90 |
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optical antennas |
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Optical antennas are devices that convert freely propagating optical radiation into localized energy, and vice versa. They enable the control and manipulation of optical fields at the nanometre scale, and hold promise for enhancing the performance and efficiency of photodetection, light emission and sensing. Although many of the properties and parameters of optical antennas are similar to their radiowave and microwave counterparts, they have important differences resulting from their small size and the resonant properties of metal nanostructures. This Review summarizes the physical properties of optical antennas, provides a summary of some of the most important recent developments in the field, discusses the potential applications and identifies the future challenges and opportunities. |
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RPLAB @ gujma @ |
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Ikuta, Rikizo; Kusaka, Yoshiaki; Kitano, suyoshi; Kato, Hiroshi; Yamamoto, Takashi; Koashi, Masato; Imoto, Nobuyuki |
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Wide-band quantum interface for visible-totelecommunication wavelength conversion |
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Journal Article |
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2011 |
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Nature Communications |
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Nat. Comm. |
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2 |
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5 |
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fromIPMRAS |
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Although near-infrared photons in telecommunication bands are required for long-distance quantum communication, various quantum information tasks have been performed by using visible photons for the past two decades. Recently, such visible photons from diverse media including atomic quantum memories have also been studied. Optical frequency down-conversion from visible to telecommunication bands while keeping the quantum states is thus required for bridging such wavelength gaps. Here we report demonstration of a quantum interface of frequency down-conversion from visible to telecommunication bands by using a nonlinear crystal, which has a potential to work over wide bandwidths, leading to a high-speed interface of frequency conversion. We achieved the conversion of a picosecond visible photon at 780 nm to a 1,522-nm photon, and observed that the conversion process retained entanglement between the down-converted photon and another photon. |
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Crespi, Andrea; Ramponi, Roberta; Osellame, Roberto; Sansoni, Linda; Bongioanni, Irene; Sciarrino, Fabio; Vallone, Giuseppe; Mataloni, Paolo |
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Integrated photonic quantum gates for polarization qubits |
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Journal Article |
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2011 |
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Nature Communications |
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Nat. Comm. |
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2 |
Issue |
566 |
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6 |
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fromIPMRAS |
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The ability to manipulate quantum states of light by integrated devices may open new perspectives both for fundamental tests of quantum mechanics and for novel technological applications. However, the technology for handling polarization-encoded qubits, the most commonly adopted approach, is still missing in quantum optical circuits. Here we demonstrate the first integrated photonic controlled-NOT (CNOT) gate for polarization-encoded qubits. This result has been enabled by the integration, based on femtosecond laser waveguide writing, of partially polarizing beam splitters on a glass chip. We characterize the logical truth table of the quantum gate demonstrating its high fidelity to the expected one. In addition, we show the ability of this gate to transform separable states into entangled ones and vice versa. Finally, the full accessibility of our device is exploited to carry out a complete characterization of the CNOT gate through a quantum process tomography. |
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