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Васильева, И. А.; Компанеец, В. В.; Красная, Ж. А.; Чижикова, З. А. |
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Проявление внутримолекулярных вибронных взаимодействий в тонкоструктурных спектрах флуоресценции и возбуждения флуоресценции полиеновых δ-диметиламинокетонов |
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Journal Article |
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2011 |
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Оптический журнал |
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Опт. ж. |
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78 |
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5 |
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3-8 |
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спектры флуоресценции; вибрационный анализ; адиабатическое гармоническое приближение; бесфононная линия; фононное крыло |
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Проведен вибрационный анализ спектров флуоресценции и возбуждения флуоресценции, полученных методом Шпольского при 4,2 K. Рассчитаны параметры внутримолекулярных взаимодействий двух δ-диметиламинокетонов. Для определения интегральных интенсивностей вибронных полос в спектрах с тонкой структурой на интенсивном сплошном фоне выполнено моделирование спектров путем представления полосы каждого из вибронных переходов бесфононной линией и фононным крылом с определенными параметрами (полуширинами, фактором Дебая–Валлера). Показано, что нарушение зеркальной симметрии в сопряженных спектрах флуоресценции и возбуждения флуоресценции этих двух соединений может быть обÑŠяснено интерференцией франк-кондоновского и герцберг-теллеровского взаимодействий. |
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RPLAB @ gujma @ |
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721 |
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Antipov, Andrei; Bell, Matt; Yasar, Mesut; Mitin, Vladimir; Scharmach, William; Swihart, Mark; Verevkin, Aleksandr; Sergeev, Andrei |
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Luminescence of colloidal CdSe/ZnS nanoparticles: high sensitivity to solvent phase transitions |
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Journal Article |
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2011 |
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Nanoscale Research Letters |
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Nan. Res. Lett. |
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6 |
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7 |
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We investigate nanosecond photoluminescence processes in colloidal core/shell CdSe/ZnS nanoparticles dissolved in water and found strong sensitivity of luminescence to the solvent state. Several pronounced changes have been observed in the narrow temperature interval near the water melting point. First of all, the luminescence intensity substantially (approximately 50%) increases near the transition. In a large temperature scale, the energy peak of the photoluminescence decreases with temperature due to temperature dependence of the energy gap. Near the melting point, the peak shows N-type dependence with the maximal changes of approximately 30 meV. The line width increases with temperature and also shows N-type dependence near the melting point. The observed effects are associated with the reconstruction of ligands near the ice/water phase transition. |
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RPLAB @ gujma @ |
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722 |
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Seleznev, V. A.; Tarkhov, M. A.; Voronov, B. M.; Milostnaya, I. I.; Lyakhno, V. Yu; Garbuz, A. S.; Mikhailov, M. Yu; Zhigalina, O. M.; Gol'tsman, G. N. |
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Deposition and characterization of few-nanometers-thick superconducting Mo-Re films |
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Journal Article |
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2008 |
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Supercond. Sci. Technol. |
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Supercond. Sci. Technol. |
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21 |
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11 |
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115006 (1 to 6) |
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We report on the fabrication and investigation of few-nanometers-thick superconducting molybdenum-rhenium (Mo-Re) films intended for use in nanowire single-photon superconducting detectors (SSPDs). Mo-Re films were deposited on sapphire substrates by DC magnetron sputtering of an Mo(60)-Re(40) alloy target in an atmosphere of argon. The films 2-10 nm thick had critical temperatures (Tc) from 5.6 to 9.7 K. HRTEM (high-resolution transmission electron microscopy) analysis showed that the films had a homogeneous structure. XPS (x-ray photoelectron spectroscopy) analysis showed the Mo to Re atom ratio to be 0.575/0.425, oxygen concentration to be 10%, and concentration of other elements to be 1%. |
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RPLAB @ gujma @ |
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723 |
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Lobanov, Y.; Tong, C.; Blundell, R.; Gol'tsman, G. |
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Title |
A study of direct detection effect on the linearity of hot electron bolometer mixers |
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Conference Article |
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2009 |
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Proc. 20th Int. Symp. Space Terahertz Technol. |
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Proc. 20th ISSTT |
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282-287 |
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HEB mixer, direct detection effect |
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We have performed a study of how direct detection affects the linearity and hence the calibration of an HEB mixer. Two types of waveguide HEB devices have been used: a 0.8 THz HEB mixer and a 1.0 THz HEB mixer which is ~5 times smaller than the former. Two independent experimental approaches were used. In the ΔG/G method, the conversion gain of the HEB mixer is first measured as a function of the bias current for a number of bias voltages. At each bias setting, we carefully measure the change in the operating current when the input loads are switched. From the measured data, we can derive the expected difference in gain between the hot and cold loads. In the second method (injection method [1]), the linearity of the HEB mixer is independently measured by injecting a modulated signal for different input load temperatures. The results of both approaches confirm that there is gain compression in the operation of HEB mixers. Based on the results of our measurements, we discuss the impact of direct detection effects on the operation of HEB mixers. |
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RPLAB @ gujma @ |
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724 |
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Lobanov, Y. V.; Tong, Cheuk-Yu E.; Hedden, A. S.; Blundell, R.; Gol'tsman, G. N. |
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Title |
Microwave-assisted슠measurement슠of the슠frequency슠response슠of슠terahertz슠HEB슠mixers슠with a슠fourier슠transform슠spectrometer |
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Conference Article |
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2010 |
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21st International Symposium on Space Terahertz Technology |
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21st ISSTT |
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420-423 |
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HEB mixer |
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We describe a novel method of operation of the HEB direct detector for use with a Fourier Transform Spectrometer. Instead of elevating the bath temperature, we have measured the RF response of waveguide HEB mixers by applying microwave radiation to select appropriate bias conditions. In our experiment, a microwave signal is injected into the HEB mixer via its IF port. By choosing an appropriate injection level, the device can be operated close to the desired operating point. Furthermore, we have shown that both thermal biasing and microwave injection can reproduce the same spectral response of the HEB mixer. However, with the use of microwave injection, there is no need to wait for the mixer to reach thermal equilibrium, so characterisation can be done in less time. Also, the liquid helium consumption for our wet cryostat is also reduced. We have demonstrated that the signalto-noise ratio of the FTS measurements can be improved with microwave injection. |
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RPLAB @ gujma @ |
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725 |
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