Bonifas, A. P., & McCreery, R. L. (2010). ‘Soft’ Au, Pt and Cu contacts for molecular junctions through surface-diffusion-mediated deposition. Nat. Nanotech., 5(8), 612–617.
Abstract: Virtually all types of molecular electronic devices depend on electronically addressing a molecule or molecular layer through the formation of a metallic contact. The introduction of molecular devices into integrated circuits will probably depend on the formation of contacts using a vapour deposition technique, but this approach frequently results in the metal atoms penetrating or damaging the molecular layer. Here, we report a method of forming 'soft' metallic contacts on molecular layers through surface-diffusion-mediated deposition, in which the metal atoms are deposited remotely and then diffuse onto the molecular layer, thus eliminating the problems of penetration and damage. Molecular junctions fabricated by this method exhibit excellent yield (typically >90%) and reproducibility, and allow examination of the effects of molecular-layer structure, thickness and contact work function.
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Ikuta, R., Kusaka, Y., Kitano, suyoshi, Kato, H., Yamamoto, T., Koashi, M., et al. (2011). Wide-band quantum interface for visible-totelecommunication wavelength conversion. Nat. Comm., 2, 5.
Abstract: Although near-infrared photons in telecommunication bands are required for long-distance quantum communication, various quantum information tasks have been performed by using visible photons for the past two decades. Recently, such visible photons from diverse media including atomic quantum memories have also been studied. Optical frequency down-conversion from visible to telecommunication bands while keeping the quantum states is thus required for bridging such wavelength gaps. Here we report demonstration of a quantum interface of frequency down-conversion from visible to telecommunication bands by using a nonlinear crystal, which has a potential to work over wide bandwidths, leading to a high-speed interface of frequency conversion. We achieved the conversion of a picosecond visible photon at 780 nm to a 1,522-nm photon, and observed that the conversion process retained entanglement between the down-converted photon and another photon.
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Knee, G. C., Simmons, S., Gauger, E. M., Morton, J. J. L., Riemann, H., Abrosimov, N. V., et al. (2012). Violation of a Leggett–Garg inequality with ideal non-invasive measurements. Nat. Comm., 3(606), 6.
Abstract: The quantum superposition principle states that an entity can exist in two different states simultaneously, counter to our 'classical' intuition. Is it possible to understand a given system's behaviour without such a concept? A test designed by Leggett and Garg can rule out this possibility. The test, originally intended for macroscopic objects, has been implemented in various systems. However to date no experiment has employed the 'ideal negative result' measurements that are required for the most robust test. Here we introduce a general protocol for these special measurements using an ancillary system, which acts as a local measuring device but which need not be perfectly prepared. We report an experimental realization using spin-bearing phosphorus impurities in silicon. The results demonstrate the necessity of a non-classical picture for this class of microscopic system. Our procedure can be applied to systems of any size, whether individually controlled or in a spatial ensemble.
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Hosseini, M., Campbell, G., Sparkes, B. M., Lam, P. K., & Buchler, B. C. (2011). Unconditional room-temperature quantum memory. Nat. Phys., 7(10), 794–798.
Abstract: Just as classical information systems require buffers and memory, the same is true for quantum information systems. The potential that optical quantum information processing holds for revolutionizing computation and communication is therefore driving significant research into developing optical quantum memory. A practical optical quantum memory must be able to store and recall quantum states on demand with high efficiency and low noise. Ideally, the platform for the memory would also be simple and inexpensive. Here, we present a complete tomographic reconstruction of quantum states that have been stored in the ground states of rubidium in a vapour cell operating at around 80 °C. Without conditional measurements, we show recall fidelity up to 98% for coherent pulses containing around one photon. To unambiguously verify that our memory beats the quantum no-cloning limit we employ state-independent verification using conditional variance and signal-transfer coefficients.
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Wei, J., Olaya, D., Karasik, B. S., Pereverzev, S. V., Sergeev, A. V., & Gershenson, M. E. (2008). Ultrasensitive hot-electron nanobolometers for terahertz astrophysics. Nature Nanotech, 3(8), 496–500.
Abstract: The submillimetre or terahertz region of the electromagnetic spectrum contains approximately half of the total luminosity of the Universe and 98% of all the photons emitted since the Big Bang. This radiation is strongly absorbed in the Earth's atmosphere, so space-based terahertz telescopes are crucial for exploring the evolution of the Universe. Thermal emission from the primary mirrors in these telescopes can be reduced below the level of the cosmic background by active cooling, which expands the range of faint objects that can be observed. However, it will also be necessary to develop bolometers – devices for measuring the energy of electromagnetic radiation—with sensitivities that are at least two orders of magnitude better than the present state of the art. To achieve this sensitivity without sacrificing operating speed, two conditions are required. First, the bolometer should be exceptionally well thermally isolated from the environment;
second, its heat capacity should be sufficiently small. Here we demonstrate that these goals can be achieved by building a superconducting hot-electron nanobolometer. Its design eliminates the energy exchange between hot electrons and the leads by blocking electron outdiffusion and photon emission. The thermal conductance between hot electrons and the thermal bath, controlled by electron–phonon interactions, becomes very small at low temperatures (10-16 WK-1 at 40 mK). These devices, with a heat capacity of 10-19 J K-1, are sufficiently sensitive to detect single terahertz photons in submillimetre astronomy and other applications based on quantum calorimetry and photon counting.
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Nozaki, K., Shinya, A., Matsuo, S., Suzaki, Y., Segawa, T., Sato, T., et al. (2012). Ultralow-power all-optical RAM based on nanocavities. Nat. Photon., 6(4), 248–252.
Abstract: Optical random-access memory (o-RAM) has been regarded as one of the most difficult challenges in terms of replacing its various functionalities in electronic circuitry with their photonic counterparts. Nevertheless, it constitutes a key device in optical routing and processing. Here, we demonstrate that photonic crystal nanocavities with an ultrasmall buried heterostructure design can solve most of the problems encountered in previous o-RAMs. By taking advantage of the strong confinement of photons and carriers and allowing heat to escape efficiently, we have realized all-optical RAMs with a power consumption of only 30 nW, which is more than 300 times lower than the previous record, and have achieved continuous operation. We have also demonstrated their feasibility in multibit integration. This paves the way for constructing a low-power large-scale o-RAM system that can handle high-bit-rate optical signals.
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Pris, A. D., Utturkar, Y., Surman, C., Morris, W. G., Vert, A., Zalyubovskiy, S., et al. (2012). Towards high-speed imaging of infrared photons with bio-inspired nanoarchitectures. Nat. Photon., 6(3), 195–200.
Abstract: Existing infrared detectors rely on complex microfabrication and thermal management methods. Here, we report an attractive platform of low-thermal-mass resonators inspired by the architectures of iridescent Morpho butterfly scales. In these resonators, the optical cavity is modulated by its thermal expansion and refractive index change, resulting in `wavelength conversion' of mid-wave infrared (3-8 µm) radiation into visible iridescence changes. By doping Morpho butterfly scales with single-walled carbon nanotubes, we achieved mid-wave infrared detection with 18-62 mK noise-equivalent temperature difference and 35-40 Hz heat-sink-free response speed. The nanoscale pitch and the extremely small thermal mass of individual `pixels' promise significant improvements over existing detectors. Computational analysis explains the origin of this thermal response and guides future conceptually new bio-inspired thermal imaging sensor designs.
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Vishveshwara, S. (2011). Topological qubits: A bit of both. Nat. Phys., 7, 450–451.
Abstract: 'Standard' qubits have been implemented in diverse physical systems. Now, so-called topological qubits are coming into the limelight, and could potentially be used for decoherence-free quantum computing. Coupling these two types of qubit might enable devices that exploit the virtues of both.
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Akalin, T. (2012). Terahertz sources: Powerful photomixers. Nat. Photon., 6(2), 81.
Abstract: An efficient continuous-wave source of terahertz radiation that combines the outputs from two near-infrared semiconductor lasers in a novel photomixer looks set to benefit applications in spectroscopy and imaging.
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Williams, B. S. (2007). Terahertz quantum-cascade lasers. Nature Photonics, 1, 517–525.
Abstract: Six years after their birth, terahertz quantum-cascade lasers can now deliver milliwatts or more of continuous-wave coherent radiation throughout the terahertz range — the spectral regime between millimetre and infrared wavelengths, which has long resisted development. This paper reviews the state-of-the-art and future prospects for these lasers, including efforts to increase their operating temperatures, deliver higher output powers and emit longer wavelengths.
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Paiella, R. (2011). Terahertz quantum cascade lasers: Going ultrafast. Nat. Photon., 5, 253–255.
Abstract: A new asynchronous coherent optical sampling method allows for the direct visualization of actively mode-locked quantum cascade laser pulses at terahertz wavelengths.
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Mineev, V. P. (2012). Superfluid helium: Order in disorder. Nat. Phys., 8, 253–254.
Abstract: Confining liquid 3He in porous silica aerogel prepared with strong anisotropy stabilizes a state of axial superfluidity.
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Gabay, M., & Triscone, J. - M. (2011). Superconductors: Terahertz superconducting switch. Nat. Photon., 5(8), 447–449.
Abstract: The use of terahertz pulses to 'gate' interlayer charge transport in a superconductor could lead to a variety of new and interesting applications.
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Billangeon, P. - M., & Nakamura, Y. (2011). Superconducting devices: Quantum cups and balls. Nat. Phys., 7(8), 594–595.
Abstract: A single microwave photon in a superposition of two states of different frequency is now demonstrated using a superconducting quantum interference device to mediate the coupling between two harmonics of a resonator. Such quantum circuits bring closer the possibility of controlling photon-photon interactions at the single-photon level.
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Haviland, D. (2010). Superconducting circuits: Quantum phase slips. Nat. Phys., 6, 565–566.
Abstract: Coulomb interactions can cause a rapid change in the phase of the wavefunction along a very narrow superconducting system. Such a phase slip at the quantum level is now measured in a chain of Josephson junctions.
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