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| Author |
Bonifas, Andrew P.; McCreery, Richard L. |
Title  |
‘Soft’ Au, Pt and Cu contacts for molecular junctions through surface-diffusion-mediated deposition |
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Journal Article |
| Year |
2010 |
Publication |
Nature Nanotechnology |
Abbreviated Journal |
Nat. Nanotech. |
| Volume |
5 |
Issue |
8 |
Pages |
612–617 |
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Virtually all types of molecular electronic devices depend on electronically addressing a molecule or molecular layer through the formation of a metallic contact. The introduction of molecular devices into integrated circuits will probably depend on the formation of contacts using a vapour deposition technique, but this approach frequently results in the metal atoms penetrating or damaging the molecular layer. Here, we report a method of forming 'soft' metallic contacts on molecular layers through surface-diffusion-mediated deposition, in which the metal atoms are deposited remotely and then diffuse onto the molecular layer, thus eliminating the problems of penetration and damage. Molecular junctions fabricated by this method exhibit excellent yield (typically >90%) and reproducibility, and allow examination of the effects of molecular-layer structure, thickness and contact work function. |
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682 |
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Ikuta, Rikizo; Kusaka, Yoshiaki; Kitano, suyoshi; Kato, Hiroshi; Yamamoto, Takashi; Koashi, Masato; Imoto, Nobuyuki |
| Title |
Wide-band quantum interface for visible-totelecommunication wavelength conversion |
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Journal Article |
| Year |
2011 |
Publication |
Nature Communications |
Abbreviated Journal |
Nat. Comm. |
| Volume |
2 |
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5 |
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fromIPMRAS |
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Although near-infrared photons in telecommunication bands are required for long-distance quantum communication, various quantum information tasks have been performed by using visible photons for the past two decades. Recently, such visible photons from diverse media including atomic quantum memories have also been studied. Optical frequency down-conversion from visible to telecommunication bands while keeping the quantum states is thus required for bridging such wavelength gaps. Here we report demonstration of a quantum interface of frequency down-conversion from visible to telecommunication bands by using a nonlinear crystal, which has a potential to work over wide bandwidths, leading to a high-speed interface of frequency conversion. We achieved the conversion of a picosecond visible photon at 780 nm to a 1,522-nm photon, and observed that the conversion process retained entanglement between the down-converted photon and another photon. |
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RPLAB @ gujma @ |
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764 |
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Knee, George C.; Simmons, Stephanie; Gauger, Erik M.; Morton, John J. L.; Riemann, Helge; Abrosimov, Nikolai V.; Becker, Peter; Pohl, Hans-Joachim; Itoh, Kohei M.; Thewalt, Mike L. W.; Briggs, G. Andrew D.; Benjamin, Simon C. |
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Violation of a Leggett–Garg inequality with ideal non-invasive measurements |
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Journal Article |
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2012 |
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Nature Communications |
Abbreviated Journal |
Nat. Comm. |
| Volume |
3 |
Issue |
606 |
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6 |
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fromIPMRAS |
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The quantum superposition principle states that an entity can exist in two different states simultaneously, counter to our 'classical' intuition. Is it possible to understand a given system's behaviour without such a concept? A test designed by Leggett and Garg can rule out this possibility. The test, originally intended for macroscopic objects, has been implemented in various systems. However to date no experiment has employed the 'ideal negative result' measurements that are required for the most robust test. Here we introduce a general protocol for these special measurements using an ancillary system, which acts as a local measuring device but which need not be perfectly prepared. We report an experimental realization using spin-bearing phosphorus impurities in silicon. The results demonstrate the necessity of a non-classical picture for this class of microscopic system. Our procedure can be applied to systems of any size, whether individually controlled or in a spatial ensemble. |
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RPLAB @ gujma @ |
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767 |
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Hosseini, M.; Campbell, G.; Sparkes, B. M.; Lam, P. K.; Buchler, B. C. |
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Unconditional room-temperature quantum memory |
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Journal Article |
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2011 |
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Nature Physics |
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Nat. Phys. |
| Volume |
7 |
Issue |
10 |
Pages |
794-798 |
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fromIPMRAS |
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Just as classical information systems require buffers and memory, the same is true for quantum information systems. The potential that optical quantum information processing holds for revolutionizing computation and communication is therefore driving significant research into developing optical quantum memory. A practical optical quantum memory must be able to store and recall quantum states on demand with high efficiency and low noise. Ideally, the platform for the memory would also be simple and inexpensive. Here, we present a complete tomographic reconstruction of quantum states that have been stored in the ground states of rubidium in a vapour cell operating at around 80 °C. Without conditional measurements, we show recall fidelity up to 98% for coherent pulses containing around one photon. To unambiguously verify that our memory beats the quantum no-cloning limit we employ state-independent verification using conditional variance and signal-transfer coefficients. |
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RPLAB @ gujma @ |
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824 |
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Wei, Jian; Olaya, David; Karasik, Boris S.; Pereverzev, Sergey V.; Sergeev, Andrei V.; Gershenson, Michael E. |
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Ultrasensitive hot-electron nanobolometers for terahertz astrophysics |
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Journal Article |
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2008 |
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Nature Nanotechnology |
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Nature Nanotech |
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3 |
Issue |
8 |
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496-500 |
| Keywords |
HEB, Ti/NbN, single terahertz photons, detection |
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The submillimetre or terahertz region of the electromagnetic spectrum contains approximately half of the total luminosity of the Universe and 98% of all the photons emitted since the Big Bang. This radiation is strongly absorbed in the Earth's atmosphere, so space-based terahertz telescopes are crucial for exploring the evolution of the Universe. Thermal emission from the primary mirrors in these telescopes can be reduced below the level of the cosmic background by active cooling, which expands the range of faint objects that can be observed. However, it will also be necessary to develop bolometers – devices for measuring the energy of electromagnetic radiation—with sensitivities that are at least two orders of magnitude better than the present state of the art. To achieve this sensitivity without sacrificing operating speed, two conditions are required. First, the bolometer should be exceptionally well thermally isolated from the environment;
second, its heat capacity should be sufficiently small. Here we demonstrate that these goals can be achieved by building a superconducting hot-electron nanobolometer. Its design eliminates the energy exchange between hot electrons and the leads by blocking electron outdiffusion and photon emission. The thermal conductance between hot electrons and the thermal bath, controlled by electron–phonon interactions, becomes very small at low temperatures (10-16 WK-1 at 40 mK). These devices, with a heat capacity of 10-19 J K-1, are sufficiently sensitive to detect single terahertz photons in submillimetre astronomy and other applications based on quantum calorimetry and photon counting. |
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1748-3387 |
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576 |
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