Abstract: Quantum networks must have the crucial ability to entangle quantum nodes. A prominent example is the quantum repeater, which allows the distance barrier of direct transmission of single photons to be overcome, provided remote quantum memories can be entangled in a heralded fashion. Here, we report the observation of heralded entanglement between two ensembles of rare-earth ions doped into separate crystals. A heralded single photon is sent through a 50/50 beamsplitter, creating a single-photon entangled state delocalized between two spatial modes. The quantum state of each mode is subsequently mapped onto a crystal, leading to an entangled state consisting of a single collective excitation delocalized between two crystals. This entanglement is revealed by mapping it back to optical modes and by estimating the concurrence of the retrieved light state. Our results highlight the potential of crystals doped with rare-earth ions for entangled quantum nodes and bring quantum networks based on solid-state resources one step closer.

Abstract: High-order nonlinear light–matter interactions in gases enable the generation of X-ray and attosecond light pulses, metrology and spectroscopy1. Optical nonlinearities in solid-state materials are particularly interesting for combining optical and electronic functions for high-bandwidth information processing2. Third-order nonlinear optical processes in silicon have been used to process optical signals with bandwidths greater than 1 GHz (ref. 2). However, fundamental physical processes for a silicon-based optical modulator in the terahertz bandwidth range have not yet been explored. Here, we demonstrate ultrafast phononic modulation of the optical index of silicon by irradiation with intense few-cycle femtosecond pulses. The anisotropic reflectivity modulation by the resonant Raman susceptibility at the fundamental frequency of the longitudinal optical phonon of silicon (15.6 THz) generates a frequency comb up to seventh order. All-optical >100 THz frequency comb generation is realized by harnessing the coherent atomic motion of the silicon crystalline lattice at its highest mechanical frequency.

Abstract: The plasmon resonance of metal nanoparticles can direct light from optical emitters in much the same way that radiofrequency antennas direct the emission from electrical circuits. Recently, rapid progress has been made in the realization of single-element antennas for optical waves. Because most of these devices are designed to optimize the local near-field coupling between the antenna and an emitter, the possibility of modifying the spatial radiation pattern has not yet received as much attention. In the radiofrequency regime, a typical antenna design for high directivity is the Yagi–Uda antenna, which essentially consists of a one-dimensional array of antenna elements driven by a single feed element. By fabricating a corresponding array of nanoparticles, similar radiation patterns can be obtained in the optical regime. Here, we present the experimental demonstration of directional control of radiation from a nano-optical Yagi–Uda antenna composed of appropriately tuned gold nanorods.

Abstract: Emission from a resonantly excited quantum emitter is a fascinating research topic within the field of quantum optics and is a useful source for different types of quantum light fields. The resonance spectrum consists of a single spectral line that develops into a triplet above saturation of the quantum emitter. The three closely spaced photon channels from the resonance fluorescence have different photon statistical signatures. We present a detailed photon statistics analysis of the resonance fluorescence emission triplet from a solid-state-based artificial atom, that is, a semiconductor quantum dot. The photon correlation measurements demonstrate both `single' and `cascaded' photon emission from the Mollow triplet sidebands. The bright and narrow sideband emission (5.9 × 106 photons per second into the first lens) can be conveniently frequency-tuned by laser detuning over 15 times its linewidth (Δv ~ 1.0 GHz). These unique properties make the Mollow triplet sideband emission a valuable light source for quantum light spectroscopy and quantum information applications, for example.

Abstract: Optical antennas are devices that convert freely propagating optical radiation into localized energy, and vice versa. They enable the control and manipulation of optical fields at the nanometre scale, and hold promise for enhancing the performance and efficiency of photodetection, light emission and sensing. Although many of the properties and parameters of optical antennas are similar to their radiowave and microwave counterparts, they have important differences resulting from their small size and the resonant properties of metal nanostructures. This Review summarizes the physical properties of optical antennas, provides a summary of some of the most important recent developments in the field, discusses the potential applications and identifies the future challenges and opportunities.