| Records |
| Author |
Parrott, Edward P. J.; Zeitler, J. Axel; Fris<cc><152>c<cc><152>ic<cc><81>, Tomislav; Pepper, Michael; Jones, William; Day, Graeme M.; Gladden, Lynn F. |
| Title |
Testing the sensitivity of terahertz spectroscopy to changes in molecular and supramolecular structure: a study of structurally similar cocrystals |
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Journal Article |
| Year |
2009 |
Publication |
Crystal Growth & Design |
Abbreviated Journal |
Crystal Growth & Design |
| Volume |
9 |
Issue |
3 |
Pages |
1452-1460 |
| Keywords |
supramolecular recognition, infrared, terahertz, IR, THz, TDS |
| Abstract |
Terahertz time-domain-spectroscopy (THz-TDS) has emerged as a versatile spectroscopic technique, and an alternative to powder X-ray diffraction in the characterization of molecular crystals. We tested the ability of terahertz spectroscopy to distinguish between chiral and racemic hydrogen-bonded cocrystals that are similar in molecular and supramolecular structure. Terahertz spectroscopy readily distinguished between the isostructural cocrystals of theophylline with chiral and racemic forms of malic acid which are almost identical in molecular structure and supramolecular architecture. Similarly, the cocrystals of theophylline with chiral and racemic forms of tartaric acid, which are similar at the molecular level but dissimilar in crystal packing, were distinguished unequivocally. The investigation of the same cocrystals using X-ray powder diffraction and Raman spectroscopy suggested that THz-TDS is comparable in sensitivity to diffraction methods and more sensitive than Raman spectroscopy to changes in cocrystal architecture. The differences in spectra acquired by THz-TDS could be further enhanced by cooling the samples to 109 K. |
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1528-7483 |
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567 |
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Pyatkov, F.; Khasminskaya, S.; Kovalyuk, V.; Hennrich, F.; Kappes, M. M.; Goltsman, G. N.; Pernice, W. H. P.; Krupke, R. |
| Title |
Sub-nanosecond light-pulse generation with waveguide-coupled carbon nanotube transducers |
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Journal Article |
| Year |
2017 |
Publication |
Beilstein J. Nanotechnol. |
Abbreviated Journal |
Beilstein J. Nanotechnol. |
| Volume |
8 |
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Pages |
38-44 |
| Keywords |
carbon nanotubes; CNT; infrared; integrated optics devices; nanomaterials |
| Abstract |
Carbon nanotubes (CNTs) have recently been integrated into optical waveguides and operated as electrically-driven light emitters under constant electrical bias. Such devices are of interest for the conversion of fast electrical signals into optical ones within a nanophotonic circuit. Here, we demonstrate that waveguide-integrated single-walled CNTs are promising high-speed transducers for light-pulse generation in the gigahertz range. Using a scalable fabrication approach we realize hybrid CNT-based nanophotonic devices, which generate optical pulse trains in the range from 200 kHz to 2 GHz with decay times below 80 ps. Our results illustrate the potential of CNTs for hybrid optoelectronic systems and nanoscale on-chip light sources. |
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Department of Materials and Earth Sciences, Technische Universitat Darmstadt, Darmstadt 64287, Germany |
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2190-4286 |
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PMID:28144563; PMCID:PMC5238692 |
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RPLAB @ kovalyuk @ |
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1109 |
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Rothermel, H.; Käufl, H. U.; Schrey, U.; Drapatz, S. |
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Thermal structure of the Martian mesosphere |
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Journal Article |
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1988 |
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Astron. Astrophys. |
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A&A |
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196 |
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296-300 |
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atmospheric temperature, carbon dioxide, infrared spectroscopy, mars atmosphere, mesosphere, emission spectra, line spectra, spatial resolution, mars, atmosphere, mesosphere, structure, thermal properties, spectra, spectroscopy, earth-based observations, temperature, patterns, infrared, polar regions, wavelengths, equipment, procedure, carbon dioxide, emissions |
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Rothermel1988 |
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450 |
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Rothermel, H.; Käufl, H. U.; Yu, Y. |
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A heterodyne spectrometer for astronomical measurements at 10 micrometers |
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Journal Article |
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1983 |
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Astron. Astrophys. |
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A&A |
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126 |
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387-392 |
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astronomical spectroscopy, infrared astronomy, infrared spectrometers, optical heterodyning, infrared telescopes, laser spectrometers, mars (planet), venus (planet) |
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453 |
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Slysz, W.; Wegrzecki, M.; Bar, J.; Grabiec, P.; Górska, M.; Latta, C.; Zwiller, V.; Pearlman, A.; Cross, A.; Korneev, A.; Kouminov, P.; Smirnov, K.; Voronov, B.; Gol’tsman, G.; Verevkin, A.; Currie, M.; Sobolewski, R. |
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Fiber-coupled quantum-communications receiver based on two NbN superconducting single-photon detectors |
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Conference Article |
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2005 |
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Proc. SPIE |
Abbreviated Journal |
Proc. SPIE |
| Volume |
5957 |
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59571K (1 to 10) |
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SSPD, SNSPD, single-photon detectors, quantum communication, quantum cryptography, superconductors, infrared optical detectors |
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We present the design and performance of a novel, two-channel single-photon receiver, based on two fiber-coupled NbN superconducting single-photon detectors (SSPDs). The SSPDs are nanostructured superconducting meanders covering an area of 100 μm2 and are known for ultrafast and efficient counting of single, visible-to-infrared photons. Their operation has been explained within a phenomenological hot-electron photoresponse model. Our receiver is intended for fiber-based quantum cryptography and communication systems, operational at near-infrared (NIR) telecommunication wavelengths, λ = 1.3 μm and λ = 1.55 μm. Coupling between the NbN detector and a single-mode optical fiber was achieved using a specially designed, micromechanical photoresist ring, positioned directly over the SSPD active area. The positioning accuracy of the ring was below 1 μm. The receiver with SSPDs was placed (immersed) in a standard liquid-helium transport Dewar and kept without interruption for over two months at 4.2 K. At the same time, the optical fiber inputs and electrical outputs were kept at room temperature. Our best system reached a system quantum efficiency of up to 0.3 % in the NIR radiation range, with the detector coupling efficiency of about 30 %. The response time was measured to be about 250 ps and was limited by our read-out electronics. The measured jitter was close to 35 ps. The presented performance parameters show that our NIR single photon detectors are suitable for practical quantum cryptography and for applications in quantum-correlation experiments. |
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SPIE |
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Rogalski, A.; Dereniak, E.L.; Sizov, F.F. |
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Infrared Photoelectronics |
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1459 |
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