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Bonifas, Andrew P.; McCreery, Richard L. |
| Title |
‘Soft’ Au, Pt and Cu contacts for molecular junctions through surface-diffusion-mediated deposition |
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Journal Article |
| Year |
2010 |
Publication |
Nature Nanotechnology |
Abbreviated Journal |
Nat. Nanotech. |
| Volume |
5 |
Issue |
8 |
Pages |
612–617 |
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Virtually all types of molecular electronic devices depend on electronically addressing a molecule or molecular layer through the formation of a metallic contact. The introduction of molecular devices into integrated circuits will probably depend on the formation of contacts using a vapour deposition technique, but this approach frequently results in the metal atoms penetrating or damaging the molecular layer. Here, we report a method of forming 'soft' metallic contacts on molecular layers through surface-diffusion-mediated deposition, in which the metal atoms are deposited remotely and then diffuse onto the molecular layer, thus eliminating the problems of penetration and damage. Molecular junctions fabricated by this method exhibit excellent yield (typically >90%) and reproducibility, and allow examination of the effects of molecular-layer structure, thickness and contact work function. |
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682 |
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Freer, Erik M.; Grachev, Oleg; Duan, Xiangfeng; Martin, Samuel; Stumbo, David P. |
| Title |
High-yield self-limiting single-nanowire assembly with dielectrophoresis |
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Journal Article |
| Year |
2010 |
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Nature Nanotechnology |
Abbreviated Journal |
Nat. Nanotech. |
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5 |
Issue |
7 |
Pages |
525–530 |
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Single-crystal nanowire transistors and other nanowire-based devices could have applications in large-area and flexible electronics if conventional top-down fabrication techniques can be integrated with high-precision bottom-up nanowire assembly. Here, we extend dielectrophoretic nanowire assembly to achieve a 98.5% yield of single nanowires assembled over 16,000 patterned electrode sites with submicrometre alignment precision. The balancing of surface, hydrodynamic and dielectrophoretic forces makes the self-assembly process controllable, and a hydrodynamic force component makes it self-limiting. Our approach represents a methodology to quantify nanowire assembly, and makes single nanowire assembly possible over an area limited only by the ability to reproduce process conditions uniformly. |
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683 |
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Konstantatos, Gerasimos; Sargent, Edward H. |
| Title |
Nanostructured materials for photon detection |
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Journal Article |
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2010 |
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Nature Nanotechnology |
Abbreviated Journal |
Nat. Nanotech. |
| Volume |
5 |
Issue |
6 |
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391–400 |
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The detection of photons underpins imaging, spectroscopy, fibre-optic communications and time-gated distance measurements. Nanostructured materials are attractive for detection applications because they can be integrated with conventional silicon electronics and flexible, large-area substrates, and can be processed from the solution phase using established techniques such as spin casting, spray coating and layer-by-layer deposition. In addition, their performance has improved rapidly in recent years. Here we review progress in light sensing using nanostructured materials, focusing on solution-processed materials such as colloidal quantum dots and metal nanoparticles. These devices exhibit phenomena such as absorption of ultraviolet light, plasmonic enhancement of absorption, size-based spectral tuning, multiexciton generation, and charge carrier storage in surface and interface traps. |
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684 |
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Wei, Jian; Olaya, David; Karasik, Boris S.; Pereverzev, Sergey V.; Sergeev, Andrei V.; Gershenson, Michael E. |
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Ultrasensitive hot-electron nanobolometers for terahertz astrophysics |
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Journal Article |
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2008 |
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Nature Nanotechnology |
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Nature Nanotech |
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3 |
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8 |
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496-500 |
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HEB, Ti/NbN, single terahertz photons, detection |
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The submillimetre or terahertz region of the electromagnetic spectrum contains approximately half of the total luminosity of the Universe and 98% of all the photons emitted since the Big Bang. This radiation is strongly absorbed in the Earth's atmosphere, so space-based terahertz telescopes are crucial for exploring the evolution of the Universe. Thermal emission from the primary mirrors in these telescopes can be reduced below the level of the cosmic background by active cooling, which expands the range of faint objects that can be observed. However, it will also be necessary to develop bolometers – devices for measuring the energy of electromagnetic radiation—with sensitivities that are at least two orders of magnitude better than the present state of the art. To achieve this sensitivity without sacrificing operating speed, two conditions are required. First, the bolometer should be exceptionally well thermally isolated from the environment;
second, its heat capacity should be sufficiently small. Here we demonstrate that these goals can be achieved by building a superconducting hot-electron nanobolometer. Its design eliminates the energy exchange between hot electrons and the leads by blocking electron outdiffusion and photon emission. The thermal conductance between hot electrons and the thermal bath, controlled by electron–phonon interactions, becomes very small at low temperatures (10-16 WK-1 at 40 mK). These devices, with a heat capacity of 10-19 J K-1, are sufficiently sensitive to detect single terahertz photons in submillimetre astronomy and other applications based on quantum calorimetry and photon counting. |
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1748-3387 |
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